國家衛生研究院 NHRI:Item 3990099045/10127
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    题名: Cobalt(II)-catalyzed aerobic oxidation of terminal-capped alkynyl alpha-cyano alkanone systems. An oxygen-mediated radical chain reaction
    其它题名: Cobalt(II)-catalyzed aerobic oxidation of terminal-capped alkynyl α-cyano alkanone systems. An oxygen-mediated radical chain reaction
    作者: Huang, JK;Wong, YC;Kao, TT;Tseng, CT;Shia, KS
    贡献者: Institute of Biotechnology and Pharmaceutical Research
    摘要: A new N-hydroxyphthalimide (NHPI)/Co(II)-catalyzed protocol, mechanistically involving a sequence of alpha-hydrogen abstraction, 5-exo-dig cyclization, oxygen capture, hydrogen transfer, and 1,4-dehydration, has been developed to facilitate aerobic oxidation of aryl-, silyl-, and alkyl-capped alkynyl alpha-cyano alkanone systems to the corresponding highly functionalized products in an effective manner, thus turning this novel chain reaction, originally occurring spontaneously in low yields, into a practical methodology.
    日期: 2016-11-18
    關聯: Journal of Organic Chemistry. 2016 Nov 18;81(22):10759-10768.
    Link to: http://dx.doi.org/10.1021/acs.joc.6b01837
    JIF/Ranking 2023: http://gateway.webofknowledge.com/gateway/Gateway.cgi?GWVersion=2&SrcAuth=NHRI&SrcApp=NHRI_IR&KeyISSN=0022-3263&DestApp=IC2JCR
    Cited Times(WOS): https://www.webofscience.com/wos/woscc/full-record/WOS:000391248800017
    Cited Times(Scopus): https://www.scopus.com/inward/record.url?partnerID=HzOxMe3b&scp=84996538523
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